This person is a member of the experimental Atomic Molecular and Optical Sciences (AMOS) Group:
"Many Particle Momentum Spectroscopy with Synchrotron Radiation and High Harmonic Laserpulses as well as Electron Impact"

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Research Interest:

The key note of my research is the investigation of many (or few, e.g. 2, 3, ..., 10) particle problems in quantum mechanics. Although the explicit motion of particles in and in-between atoms and molecules is not subject of this very well tested and successful theory (instead a probability density function is introduced which obscures the appreciation), it is the correlated dynamics of electrons which for instance is responsible for the formation of Cooper-pairs, e.g. the elements of the fractionate Hall effect and heavy Fermi-particles.

However, the main idea or focus is to uncover the entangled motion of electrons in unperturbed atoms, molecules, clusters and surfaces. Or in other words to answer the question: What makes the collective motion in bound many particle systems tick ? Since it is not possible to peer inside an atom, molecule or any other many particle system without altering it, it is very difficult to cotton on to this important question.

The fundamental idea is to probe an atom or molecule (or surface) in a manner that preserves most of its internal motion which can be detected in a kinematically complete experiment, e.g. an experiment where all final state momentum vectors of all particles are known with 4 solid angle at best (in most cases without knowledge about the spin).

The key value in the description of the dynamics of these complex systems is the three dimensional momentum vector of each particle. Therefore a device is needed that visualizes the trajectories of all particles in the 'explosion' (e.g. ionization or fragmentation) of the target. Once all momentum vectors of the outcome are obtained, highly differential cross sections (triple, quadruple or higher differential in angles and energies) reveal the information of the entangled motion of the particles. The coincident momentum spectroscopy of electrons and recoiling ions, which has been used by the applicant very successfully in the past and which is known as COLd Target Recoil Ion Momentum Spectroscopy COLTRIMS or reactions microscopy (described below), is able to elucidate what is going on here.

Figure 1: Schematically drawing of the momentum spectrometer: The deuterium molecules, prepared in a supersonic jet going from the bottom to the top, are intersected with the pulsed photon beam in the middle of the copper rings which define a homogenous electrical field. The big coils represent a Helmholtz pair which establishes a homogenous magnetic field in parallel to the spectrometer axis. The nuclei are guided to a position sensitive detector to the left while the electrons get spiraled to the right (due to their low mass in the magnetic field).




As already mentioned above, peering in a microscopic system like atoms and molecules with particle beams and electromagnetic waves results in exciting and fragmenting or ionizing the target. Once bonds are broken an explosion of the system is triggered which is superimposing the internal motion of the initial state. This is due to Coulomb repulsion or post collision interaction (or post absorption interaction in case of photoionization processes) and is influenced by selection rules as well as momentum and energy conservation laws etc. To track down which structure of the complex emission patterns is due to the initial dynamics of the entangled motion of the particles, the knowledge about final state interactions and their associated highly differential cross sections is indispensable: Ionization mechanisms (such as TS1, TS2, GSC, shake-off for the double ionization), post collision (or post absorption) interaction between the fragments (as well as diffraction and interference), and internal properties of the binding (like symmetry effects, the inter-nuclear separation of a molecule at the time of photo ionization or bond-angles for instance) have to be studied and have to be "subtracted" (resp. isolated) in momentum space in order to see the finger-print of the dynamics of the initial state.

But investigating these final state interactions and internal properties of the systems as well as ionization mechanisms is much more than just a necessary condition: Once atoms and molecules absorb enough energy by probing the target with particle beams and/or electromagnetic waves, bonds can be broken and ions can form, allowing neutral and charged constituents to react with their neighbors. These processes occur everywhere, from car engines to industrial chemical plants. Ionization processes also occur naturally in earth's upper atmosphere, driven by the sun's energy, and are the mechanisms responsible for radiation damage to our bodies. In general, the more en-ergy that is absorbed - either from light or through a collision with another energetic particle - the greater the number of possible reaction pathways and the greater the 'damage' done to the system itself and its nearest neighbors. This is a major field of research and momentum spectroscopy can help to answer fundamental questions which play an important role in many branches of physics and chemistry as well as micro biology.

For an illustration of my research goals and some project ideas please use the following link (talk as PDF-file): Overview

Publications:

#	AUTHOR	THESES
A.	Th. Weber	Impulstransfer in Proton-Heliumstößen untersucht mit hochauflösender Rückstoßionenimpulsspektroskopie Diplom-Thesis at the Institut für Kernphysik Frankfurt of Johann-Wolfgang-Goethe Universität Frankfurt a.M., (1999) ThorstenWeber-1999-2ndEdition.pdf
B.	Th. Weber	Untersuchung der verschränkten Bewegung freier Elektronenpaare emittiert aus Ein- und Zweizentren Coulomb-Potentialen in Photoabsorptionsprozessen PhD-Thesis at the Institut für Kernphysik Frankfurt of Johann-Wolfgang-Goethe Universität Frankfurt a.M., (2003) Thorsten_Weber_2003screen.pdf




#	AUTHORS	ARTICLE IN PAPER/BOOK
1.	R. Dörner, ..., T. Weber et al.	Kinematically Complete Experiments using Cold Target Recoil Ion Momentum Spectroscopy Nucl. Instr. Meth., B 124, (1997), 225 Doerner_97_NIM_B.pdf
2.	B. Bapat, ..., Th. Weber et al.	Double ionization of helium by fast fully stripped ions Physica Scripta, T808, (1999), 351 - 353 Bapat_99_PhysScr.pdf
3.	B. Krässig, ..., Th. Weber et al.	Compton double ionization of helium in the region of the cross-section maximum Phys. Rev. Lett., 83, (1999), 53 - 56 Kraessig_99_PRL.pdf
4.	B. Bapat, ..., Th. Weber et al.	Double ionization of helium in fast ion collisions: The role of momentum transfer J. Phys. B: At. Mol. Opt. Phys., 32, (1999), 1859 - 1872 Bapat_99_JPB.pdf
5.	Kh. Khayyat, Th. Weber et al.	Differential cross sections in antiproton- and proton-helium collisions J. Phys. B: At. Mol. Opt. Phys., 32, (1999), Letter to the Editor, L73 - L79 Khayyat_99_JPB.pdf
6.	L. Spielberger,..., Th. Weber et al.	Cross-section ratio of double to single ionization of helium by Compton scattering of 40-100 keV X-rays Phys. Rev. A, 59, (1999), 371 - 379 Spielberger_98_PRA.pdf
7.	H. Schmidt-Böcking, ..., Th. Weber et al.	Cold target helium recoil ion momentum imaging: Understanding correlated electron motion in the double ionisation process Australian Journal of Physics, 52, (1999), 523 - 535 SchmidtBoecking_99_AustrJournPhys.pdf
8.	Th. Weber et al.	Recoil-Ion Momentum Distributions for Single and Double Ionization of Helium in Strong Laser Fields Phys. Rev. Lett., 84, (2000), 443 - 446 Weber_PRL_2000.pdf
9.	Th. Weber et al.	Sequential and nonsequential contributions to double ionization in strong laser fields J. Phys. B: At. Mol. Opt. Phys., 33, (2000), L127 - L133 Weber_JPB_2000_A.pdf
10.	Th. Weber et al.	Correlated Electron Emission in Multiphoton Double Ionization Nature, Vol. 405, 8 June, (2000), 658 Weber_Nature_2000.pdf
11.	Th. Weber et al.	Kinematically complete investigation of momentum transfer for single ionization in fast proton-helium collisions J. Phys. B: At. Mol. Opt. Phys., 33, (2000), 3331 - 3344 Weber_JPB_2000_B.pdf
12.	Th. Weber et al.	Abrupt rise of the longitudinal recoil ion momentum distribution for ionizing collisions Phys. Rev. Lett., 86, (2001), 224 - 227 Weber_PRL_2001.pdf
13.	V. Mergel, ..., Th. Weber et al.	Strong Correlations in the He ground state momentum wave function - observed in the fully differential momentum distributions for the four particle p+He transfer ionization process Phys. Rev. Lett., 86, (2001), 2257 - 2260 Mergel_PRL_2001.pdf
14.	Y. Muramatsu, ..., Th. Weber et al.	Bent and linear geometries of Renner-Teller pair states in CO2 probed by triple-ion-coincidence momentum imaging Surface Rev. Lett., 9, (2002), 93 - 97 Muramatsu_SurfRevLett_2002.html
15.	Th. Weber et al.	Atomic Dynamics in Single and Multi Photon Double Ionization: An Experimental Comparision Optics Express, 8, (2001), 368 - 376 Weber_OptExp_2001.pdf
16.	A. Landers, Th. Weber et al.	Photoelectron Diffraction Mapping: Molecules Illuminated from Within Phys. Rev. Lett., 86, (2001), 013002-1 Landers_PRL_2001.pdf
17.	Th. Weber et al.	K-Shell Photoionization of CO and N2: Is there a link between photoelectron and angular distribution and molecular decay dynamics ? J. Phys. B: At. Mol. Opt. Phys., 34, (2001), 3669 Weber_JPB_2001.pdf
18.	M. Weckenbrock, ..., Th. Weber et al.	Experimental Evidence for Electron Repulsion in Multiphoton Double Ionization J. Phys. B: At. Mol. Opt. Phys, 34, (2001), L449 - L455 Weckenbrock_PRL_2001.pdf
19.	Y. Muramatsu, ..., Th. Weber et al.	Direct Probe of the Bent and Linear Geometries of the Core-Excited Renner-Teller Pair States Probed by the Triple-Ion-Coincidence Momentum Imaging Technique Phys. Rev. Lett., 88, (2002), 133002-1 Muramatsu_PRL_2002.pdf
20.	R. Dörner, ..., Th. Weber et al.	Many Particles Quantum Dynamics in Atomic and Molecular Fragmentation "From Atoms to Molecules", Ed.: V.P. Shevelko and J. Ullrich, Springer Verlag, (2002) Doerner_ShevelkoBook_2002.pdf
21.	T. Jahnke, Th. Weber et al.	Circular Dichrosim in K-shell ionization from Fixed-in-Space CO and N2 Molecules Phys. Rev. Lett., 88, (2002), 073002-1, front page Jahnke_PRL_2002.pdf
22.	R. Dörner, ..., Th. Weber et al.	Multiple Ionization in Strong Laser Fields "Advances in Atomic and Molecular Physics 2002", Volume 48 Ed.: B. Bederson and H. Walther, Academic Press, Amsterdam, (2002) Doerner_BedersonBook_2002.pdf
23.	F. Afaneh, ..., Th. Weber et al.	Must saddle point electrons always ride on the saddle ? J. Phys. B: At. Mol. Opt. Phys., 35, (2002), Letter to the Editor, L229 - L235 Afaneh_JPB_2002.pdf
24.	A. Knapp, ..., Th. Weber et al.	Mechanisms of Photo Double Ionization of Helium by 530 eV Photons Phys. Rev. Lett., 89, (2002), 033004-1 Knapp_PRL_2002.pdf
25.	O. Jagutzki, ..., Th. Weber et al.	Multiple hit readout of a microchannel plate detector with a three layer delay-line anode IEEE Transactions on Nuclear Science, 49, (2002), 2477 - 2483 Jagutzki_IEEE_2002.pdf
26.	H. Schmidt-Böcking, ..., Th. Weber et al.	Revealing the non-s2 contributions in the momentum wave function of ground state He Europhys. Rev. Lett., 62, (2002), 477 - 483 SchmidtBoecking_EPL_2003.pdf
27.	H. Schmidt-Böcking, ..., Th. Weber et al.	Fast p-He transfer ionization processes: An observation window to reveal the non-s2 con-tributions in the momentum wave function of ground state He "Many-Particle Quantum Dynamics in Atomic und Molecular Fragmentation", Ed.: V.P. Shevelko and J. Ullrich, Springer Verlag, (2002) liable with costs
28.	Th. Weber et al.	Auger electron emission from fixed in space CO Phys. Rev. Lett, 90, (2002), 153003-1 Weber_PRL_2003.pdf
29.	A. Knapp, ..., Th. Weber et al.	Energy sharing and asymmetry parameters for photo double ionization of Helium 100 eV above threshold in single particle and Jacobi coordinates J. Phys. B: At. Mol. Opt. Phys., 235, (2002), L521 - L526 Knapp_JPB_2002.pdf
30.	T. Osipov, ..., Th. Weber et al.	Photoelectron-Photoion momentum Spectroscopy as a Clock for Chemical Rearrange-ments: Isomerization of the Di-Cation of Acetylene to the Vinylidene Configuration Phys. Rev. Lett., 90, (2003), 233002-1 Osipov_PRL_2003.pdf
31.	R. Dörner, ..., Th. Weber et al.	Double Ionization by One and Many Photons Journal of Radiation Physics and Chemistry, 70, (2004), 191-206 Doerner_JRPC_2004.pdf
32.	H. Schmidt-Böcking, ..., Th. Weber et al.	Dynamics of ionization processes studied with the COLTRIMS method: New insight into e-e correlation Radiation Physics and Chemistry, 68, (2003), 4150 SchmidtBoecking_JRPC_2004.pdf
33.	Th. Weber et al.	Fully differential cross sections for photo double ionization of fixed in space D2 Phys. Rev. Lett., 92, (2004), 163001-1 Weber_PRL_2004.pdf
34.	T. Jalowy, Th. Weber et al.	Initial velocity of secondary ions from XY-TOF technique, simultaneous calibration by residual gas ionization International Journal of Mass Spectrometry, 231, (2004), 51 - 58 Jalowy_IJMS_2004.pdf
35.	M. Hattass, ..., T. Weber et al.	A 2pi Spectrometer for Electron-Electron Coincidence Studies on Surfaces Review of Scientific Instruments, 75, No. 7, (2004), 2373 - 2378 Hattass_RSI_2004.pdf
36.	H. Schmidt-Boecking, ..., Th. Weber et al.	Many-particle dynamics in atomic and molecular physics investigated with the COLTRIMS-technique: New inside into e-e- correlation Nucl. Ph. A, 737, (2004), p. 306 - 313 SchmidtBoecking_NPA_2004.pdf
37.	M. Weckenbrock, ..., Th. Weber et al.	Fully differential rates for multiphoton double ionization Phys. Rev. Lett., 92, (2004), 213002-1, front page Weckenbrock_PRL_2004.pdf
38.	L.Ph.H. Schmidt, ..., Th. Weber et al.	Fully Differential Study of Transfer Ionization Processes - a View into Correlated Many Particle Dynamics Physica Scripta, Vol. T110, (2004), 379 - 383 Schmidt_PhysScr_2004.pdf
39.	A. Czasch, ..., Th. Weber et al.	Doubly Excited States in Helium Close to the Double Ionization Threshold: Angular and Energy Resolved Partial Cross Sections Physica Scripta, Vol. T110, (2004), 141 - 143 Czasch_PhysScr_2004.pdf
40.	T. Jahnke, Th. Weber et al.	Multicoincidence studies of photo and Auger electrons from fixed-in-space molecules using the COLTRIMS technique Journal of Electron Spectroscopy and Related Phenomena, 141, (2004), 229 - 238 Jahnke_JES_2004.pdf
41.	Th. Weber et al.	Complete Photo-fragmentation of the Deuterium Molecule Nature, 431, (2004), 437 - 440, Erratum: Nature, Vol. 443, (2006), 1014 Weber_Nature_2004.pdf
42.	N. Saito, ..., Th. Weber et al.	Deformation, nuclear motion and fragmentation of core-excited CO2 probed by multiple-ion coincidence momentum imaging J. of Elec. Spec. and Rel. Phen., 141, (2004), 183 - 193 Saito_JESRP_2004.pdf
43.	D. Zeidler, ..., Th. Weber et al.	Fully differential rates for femtosecond multiphoton double ionization of neon Photonics North 2004: Photonic Applications in Tele-communications, Sensors, Software, and Lasers, edited by J. Armitage, R. Lessard, G. Lampropoulos, Proc. of SPIE Vol. 5579 (SPIE, Bellingham, WA, 2004), page 708 ff Zeidler_SPIE_2005.pdf
44.	A. Knapp, ..., Th. Weber et al.	Photo double ionization of helium 100 eV and 450 eV above threshold: I. Linearly polarized light J. Phys. B: At. Mol. Opt. Phys., 38, (2005), 615-633 Knapp_JPB_2005_I.pdf
45.	A. Knapp, ..., Th. Weber et al.	Photo double ionization of helium 100 eV and 450 eV above threshold: II. Circularly polarized light J. Phys. B: At. Mol. Opt. Phys., 38, (2005), 635-643 Knapp_JPB_2005_II.pdf
46.	A. Knapp, ..., Th. Weber et al.	Photo double ionization of helium 100 eV and 450 eV above threshold: III. Gerade and ungerade amplitudes and their relative phases J. Phys. B: At. Mol. Opt. Phys., 38, (2005), 645-657 Knapp_JPB_2005_III.pdf
47.	A. Czasch, ..., Th. Weber et al.	Photo induced multiple fragmentation of atoms and molecules: Dynamics of Cou-lombic many-particle systems studied with the COLTRIMS reaction microscope Phys. Lett. A, 347, (2005), 95 - 102 Czasch_PhysLettA_2005.pdf
48.	T. Osipov, ..., Th. Weber et al.	Photon–ion collisions and molecular clocks J. of Mod. Opt., 52, No. 2-3, (2005), 439 - 451 Osipov_JouModOptics_2005.pdf
49.	H. Schmidt-Boecking, ..., Th. Weber et al.	Many-particle fragmentation processes in atomic and molecular physics – new insight into the world of correlation Nucl. Instr. Meth., B 233, (2005), 3 - 11 SchmidtBoecking_NIMB_2005.pdf
50.	Thorsten Weber	Verschränkte Elektronenbewegung in Deuteriummolekülen Phys. Unserer Zeit, 36. Jahrgang, Nr. 1, (2005), 6 - 7 Weber_Physik_in_unserer_Zeit_2005.pdf
51.	A. Czasch, ..., Th. Weber et al.	Partial Photoionization Cross Sections and Angular Distributions for Double Excitation of Helium up to the N 13 Threshold Phys. Rev. Lett., 95, (2005), 243003-1 to 4, Erratum: Phys. Rev. Lett., 97, (2006), 259902-1 to 4 Czasch_PRL_2005.pdf
52.	K. Hosaka, ..., Th. Weber et al.	Nondipole effects in the angular distribution of photoelectrons from the C K shell of the CO molecule Phys. Rev. A, 73, (2006), 022716-1 to 8 Hosaka_PRA_2005.pdf
53.	A. Staudte, ..., Th. Weber et al.	Attosecond Strobing of Two-Surface Population Dynamics in Dissociating H2+ Phys. Rev. Lett., 98, (2007), 073003-1 to 4 Staudte_PRL_a_2007.pdf
54.	F. Martin, ..., Th. Weber et al.	Photo induced multiple fragmentation of atoms and molecules: Dynamics of Cou-lombic many-particle systems studied with the COLTRIMS reaction microscope Science, 315, (2007), 629 - 633 Martin_Science_2007.pdf
55.	R. Moshammer, ..., Th. Weber et al.	Few-Photon Multiple Ionization of Ne and Ar by Strong Free-Electron-Laser Pulses Phys. Rev. Lett., 98, (2007), 203001-1 to 4 and Virtual Journal of Ultrafast Science, June 2007 Moshammer_PRL_2007.pdf
56.	A. Czasch, ..., Th. Weber et al.	Reply to L. Malegat, Phys. Rev. Lett. 98,(2007), 109301 Phys. Rev. Lett., 98, (2007), 109302-1 to 4 Czasch_PRL_2007.pdf
57.	L. Schmidt, ..., Th. Weber et al.	Imaging of continuum states of the He2++ quasimolecule Phys. Rev. A, 76, (2007), 012703-1 to 9 Schmidt_PRA_2007.pdf
58.	D. Akoury, ..., Th. Weber et al.	The Simplest Double Slit: Interference and Entanglement in Double Photoionization of H2 Science, 318, (2007), 949 - 952 Akoury_Science_2007.pdf
59.	T. Jahnke, ..., Th. Weber et al.	Experimental Separation of Virtual Photon Exchange and Electron Transfer in Interatomic Coulombic Decay of Neon Dimers Phys. Rev. Lett., 99, (2007), 153401-1 to 4 Jahnke_PRL_2007.pdf
60.	A. Staudte, ..., Th. Weber et al.	Binary and Recoil Collisions in Strong Field Double Ionization of Helium Phys. Rev. Lett., 99, (2007), 263002-1 to 4 Staudte_PRL_b_2007.pdf
61.	K. Kreidi, ..., Th. Weber et al.	Interference in the Collective Electron Momentum in Double Photoionization of H2 Phys. Rev. Lett., 100, (2008), 133005-1 to 4 Kreidi_PRL_2008.pdf
62.	M. Schoeffler, ..., Th. Weber et al.	Ultrafast Probing of Core Hole Localization in N2 Science, 320, (2008), 920 - 923 Schoeffler_Science_2008.pdf
63.	Y. Morishita, ..., Th. Weber et al.	Evidence of interatomic Coulombic decay in ArKr after Ar 2p Auger decay J. Phys. B: At. Mol. Opt. Phys., 41, (2008), 025101 Morishita_JPB_2008.pdf
64.	K. Ueda, ..., Th. Weber et al.	Interatomic Coulombic decay following the Auger decay: Experimental evidence in rare-gas dimers J. Elec. Spec.. Relat. Phenom., 166-167, (2008,) 3-10 Ueda_JESRP_2008.pdf
65.	T. Osipov, ..., Th. Weber et al.	Fragmentation pathways for selected electronic states of the acetylene dication J. Phys. B: At. Mol. Opt. Phys., 41, (2008), 091001 Osipov_JPB_2008.pdf
66.	K. Kreidi, ..., Th. Weber et al.	Localization of inner-shell photoelectron emission and interatomic Coulombic decay in Ne2 J. Phys. B: At. Mol. Opt. Phys., 41, (2008), 101002 Kreidi_JPB_2008.pdf
67.	K. Kreidi, ..., Th. Weber et al.	Relaxation processes following 1s photoionization and Auger decay in Ne2 Phys. Rev. A, 78, (2008), 043422 Kreidi_PRA_2008.pdf.pdf
68.	M. Schoeffler, ..., Th. Weber et al.	Photo-double-ionization of H2: Two-center interference and its dependence on the internuclear distance Phys. Rev. A, 78, (2008), 013414-1 to 5 Schoeffler_PRA_2008.pdf
69.	K. Kreidi, ..., Th. Weber et al.	Single photon double ionization of H2 by circularly polarized photons at a photon energy of 160 eV Eur. Phys. J. Special Topics, 169, (2009), 109-116 Kreidi_EPJ_2009.pdf
70.	A.L. Landers, ..., Th. Weber et al.	Angular Correlation between Photoelectrons and Auger Electrons from K-Shell Ionization of Neon Phys. Rev. Lett., 102, (2009), 223001 Landers_PRL_2009.pdf
71.	K. Kreidi, ..., Th. Weber et al.	Photo- and Auger-Electron Recoil Induced Dynamics of Interatomic Coulombic Decay Phys. Rev. Lett., 103, (2009), 033001 Kreidi_PRL_2009.pdf
72.	F.P. Sturm, ..., Th. Weber et al.	Photo- and Auger Electron Angular Distributions of Fixed-in-Space CO2 Phys. Rev. A, 80, (2009), 032506 Sturm_PRA_2009.pdf
73.	H. Adaniya, ..., Th. Weber et al.	Imaging the Molecular Dynamics of Dissociative Electron Attachment to Water Phys. Rev. Lett., 103, (2009), 233201 Adaniya_PRL_2009.pdf
74.	N.A. Cherepkov, ..., Th. Weber et al.	Separation of Auger transitions into different repulsive states after K-shell photoionization of N2 molecules Physical Review A, 80, (2009), 051404 Cherepkov_PRA_2009.pdf
75.	T.Y. Osipov, ..., Th. Weber et al.	Formation of inner-shell autoionizing CO+ states below the CO++ threshold Accepted for publication in Physical Review A, (2010) Osipov_PRA_2010.pdf
76.	T.Y. Osipov, ..., Th. Weber et al.	Carbon K-shell photoionization of fixed-in-space C2H4 Submitted for publication in Physical Review A, (2010) XXX_XXX_2010.pdf

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Access Provider and responsible Contact Person: Thorsten Weber


Rapid communication via Phone: Tel.: 1 (510) 486 5588


Electronic Mail: TWeber@lbl.gov


Postal Address: Lawrence Berkelely National Lab, 1 Cyclotron Road, Berkeley, CA-94720, USA


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